Synthesis of luminescent silicon clusters by spark ablation

Abstract

The synthesis of luminescent nanometer-scale Si clusters by spark ablation from a crystalline Si substrate is described. The cluster source, described in the text, generates clusters in a flowing Ar stream at atmospheric pressure. Electron microscopy reveals that the clusters have diameters in the 2-4 nm size range. The luminescence spectra of the clusters, similar to that of porous Si, are presented.

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