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Published November 10, 2008 | Accepted Version
Journal Article Open

Ping-Pong Electron Transfer through DNA

Abstract

Herein we describe a novel Ir system that is able to promote the reduction of pyrimidine bases from a distance without the presence of an external quencher. Instead, DNA-mediated ET is triggered by DNA-mediated HT. Thus, photoactivation of these Ir assemblies results in both a forward and a reverse pattern for charge migration, which we term ping-pong electron transfer through DNA (Scheme 1).

Additional Information

© 2008 Wiley-VCH. Received: July 22, 2008. Published online: October 16, 2008. This work was supported by the NIH (GM49216).

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