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Published March 2023 | Supplemental Material
Journal Article Open

Non-equilibrium spectral phase transitions in coupled nonlinear optical resonators

Abstract

Coupled systems with multiple interacting degrees of freedom provide a fertile ground for emergent dynamics, which is otherwise inaccessible in their solitary counterparts. Here we show that coupled nonlinear optical resonators can undergo self-organization in their spectrum leading to a first-order phase transition. We experimentally demonstrate such a spectral phase transition in time-multiplexed coupled optical parametric oscillators. We switch the nature of mutual coupling from dispersive to dissipative and access distinct spectral regimes of the parametric oscillator dimer. We observe abrupt spectral discontinuity at the first-order transition point. Furthermore, we show how non-equilibrium phase transitions can lead to enhanced sensing, where the applied perturbation is not resolvable by the underlying linear system. Our approach could be exploited for sensing applications that use nonlinear driven-dissipative systems, leading to performance enhancements without sacrificing sensitivity.

Additional Information

© 2023 Springer Nature. We thank S. Jahani and M. Gyun Suh for helpful discussions. We acknowledge support from ARO grant no. W911NF-18-1-0285 (A.M.), AFOSR award FA9550-20-1-0040 (A.M.), NSF grant nos. 1846273 (A.M.) and 1918549 (A.M.), and NASA. We wish to thank NTT Research for their financial and technical support. Contributions. A.R. and A.M. conceived the idea. A.R. performed the experiments with help from R.N. A.R. developed the theory and performed the numerical simulations. C.L. fabricated the PPLN waveguide used in the experiment with the supervision of M.F. A.R. and A.M. wrote the manuscript with input from all authors. A.M. supervised the project. Data availability. Source data are available for this paper and can be found at https://doi.org/10.6084/m9.figshare.21252147. All other data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request. Code availability. The codes that support the findings of this study are available from the corresponding author upon reasonable request. The authors declare no competing interests.

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August 22, 2023
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October 25, 2023