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Published March 8, 2022 | Supplemental Material + Published
Journal Article Open

Dual-field-of-view high-spectral-resolution lidar: Simultaneous profiling of aerosol and water cloud to study aerosol–cloud interaction

Abstract

Aerosol–cloud interaction (ACI) is complex and difficult to be well represented in current climate models. Progress on understanding ACI processes, such as the influence of aerosols on water cloud droplet formation, is hampered by inadequate observational capability. Hitherto, high-resolution and simultaneous observations of diurnal aerosol loading and cloud microphysical properties are challenging for current remote-sensing techniques. To overcome this conundrum, we introduce the dual-field-of-view (FOV) high-spectral-resolution lidar (HSRL) for simultaneously profiling aerosol and water cloud properties, especially water cloud microphysical properties. Continuous observations of aerosols and clouds using this instrument, verified by the Monte Carlo simulation and coincident observations of other techniques, were conducted to investigate the interactions between aerosol loading and water cloud microphysical properties. A case study over Beijing highlights the scientific potential of dual-FOV HSRL to become a significant contributor to the ACI investigations. The observed water cloud profiles identify that due to air entrainment its vertical structure is not perfectly adiabatic, as assumed by many current retrieval methods. Our ACI analysis shows increased aerosol loading led to increased droplet number concentration and decreased droplet effective radius—consistent with expectations—but had no discernible increase on liquid water path. This finding supports the hypothesis that aerosol-induced cloud water increase caused by suppressed rain formation can be canceled out by enhanced evaporation. Thus, these observations obtained from the dual-FOV HSRL constitute substantial and significant additions to understanding ACI process. This technique is expected to represent a significant step forward in characterizing ACI.

Additional Information

© 2022 the Author(s). Published by PNAS. This open access article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND). Received: June 10, 2021. Accepted: January 22, 2022. Published online: March 2, 2022. Published in issue: March 8, 2022. This article is a PNAS Direct Submission. We specially acknowledge Dr. Daniel Rosenfeld (Hebrew University of Jerusalem) and Dr. Zongyin Yang (Zhejiang University) for their valuable comments to improve the manuscript. We acknowledge Dr. Lei Bi and Dr. Wushao Lin (Zhejiang University) for their great help on the cloud depolarization simulations. This study was supported by the National Key Research and Development Program of China (2016YFC0200700), the National Natural Science Foundation of China (41775023, 41925022), the Excellent Young Scientist Program of Zhejiang Provincial Natural Science Foundation of China (LR19D050001), Fundamental Research Funds for the Central Universities (2019FZJD011), the State Key Laboratory of Modern Optical Instrumentation Innovation Program (MOI2018ZD01), and the Belarusian State Research Program Photonics and Electronics for Innovations. Data Availability.The VIIRS data in Fig. 3 D and E can be freely accessed from https://ncc.nesdis.noaa.gov/VIIRS/. The ACI index data in Fig. 4G can be found in the corresponding references cited in this manuscript. All other study data are included in the article and/or SI Appendix.

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Additional details

Created:
August 22, 2023
Modified:
October 23, 2023