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Published November 12, 2021 | Submitted + Supplemental Material + Published
Journal Article Open

Direct Observation of Collective Electronuclear Modes about a Quantum Critical Point

Abstract

We directly measure the low energy excitation modes of the quantum Ising magnet LiHoF₄ using microwave spectroscopy. Instead of a single electronic mode, we find a set of collective electronuclear modes, in which the spin-1/2 Ising electronic spins hybridize with the bath of spin-7/2 Ho nuclear spins. The lowest-lying electronuclear mode softens at the approach to the quantum critical point, even in the presence of disorder. This softening is rapidly quenched by a longitudinal magnetic field. Similar electronuclear structures should exist in other spin-based quantum Ising systems.

Additional Information

© 2021 American Physical Society. Received 12 January 2021; revised 12 July 2021; accepted 13 October 2021; published 12 November 2021. The experimental work at Caltech was supported by the U.S. Department of Energy Basic Energy Sciences Award No. DE-SC0014866. P. C. E. S. acknowledges support at Caltech from Simons Foundation Grant No. 568762 and National Science Foundation Grant No. PHY-1733907. Theoretical work at UBC was supported by the National Sciences and Engineering Research Council of Canada, No. RGPIN-2019-05582.

Attached Files

Published - PhysRevLett.127.207202.pdf

Submitted - 2101.05143.pdf

Supplemental Material - 21.09.02_LiHo-PRL-suppInfo.pdf

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August 20, 2023
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