Percolating through networks of random thresholds: Finite temperature electron tunneling in metal nanocrystal arrays

Abstract

We investigate how temperature affects transport through large networks of nonlinear conductances with distributed thresholds. In monolayers of weakly coupled gold nanocrystals, quenched charge disorder produces a range of local thresholds for the onset of electron tunneling. Our measurements delineate two regimes separated by a crossover temperature T^∗. Up to T^∗ the nonlinear zero-temperature shape of the current-voltage curves survives, but with a threshold voltage for conduction that decreases linearly with temperature. Above T^∗ the threshold vanishes and the low-bias conductance increases rapidly with temperature. We develop a model that accounts for these findings and predicts T^∗.

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