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Published March 6, 2012 | Supplemental Material + Published
Journal Article Open

Process-evaluation of tropospheric humidity simulated by general circulation models using water vapor isotopologues: 1. Comparison between models and observations

Abstract

The goal of this study is to determine how H_2O and HDO measurements in water vapor can be used to detect and diagnose biases in the representation of processes controlling tropospheric humidity in atmospheric general circulation models (GCMs). We analyze a large number of isotopic data sets (four satellite, sixteen ground-based remote-sensing, five surface in situ and three aircraft data sets) that are sensitive to different altitudes throughout the free troposphere. Despite significant differences between data sets, we identify some observed HDO/H_2O characteristics that are robust across data sets and that can be used to evaluate models. We evaluate the isotopic GCM LMDZ, accounting for the effects of spatiotemporal sampling and instrument sensitivity. We find that LMDZ reproduces the spatial patterns in the lower and mid troposphere remarkably well. However, it underestimates the amplitude of seasonal variations in isotopic composition at all levels in the subtropics and in midlatitudes, and this bias is consistent across all data sets. LMDZ also underestimates the observed meridional isotopic gradient and the contrast between dry and convective tropical regions compared to satellite data sets. Comparison with six other isotope-enabled GCMs from the SWING2 project shows that biases exhibited by LMDZ are common to all models. The SWING2 GCMs show a very large spread in isotopic behavior that is not obviously related to that of humidity, suggesting water vapor isotopic measurements could be used to expose model shortcomings. In a companion paper, the isotopic differences between models are interpreted in terms of biases in the representation of processes controlling humidity.

Additional Information

© 2012 American Geophysical Union. Received 26 July 2011; revised 29 November 2011; accepted 30 December 2011; published 6 March 2012. The ACE mission is supported mainly by the Canadian Space Agency. Level-1b data of MIPAS have been provided by ESA. U.S. funding for TCCON comes from NASA's Terrestrial Ecology Program, the Orbiting Carbon Observatory project and the DOE/ARM Program. The Lauder TCCON measurements are funded by New Zealand Foundation for Research, Science and Technology contracts CO1X0204 and CO1X0406. We thank J. Robinson, who acquires the FTS data at the Lauder site, and B. Connor, who was instrumental in setting up the Lauder TCCON measurements. TCCON measurements at Wollongong and Darwin are supported by Australian Research Council grant DP0879468. The Karlsruhe FTIR experiment has been funded by the Federal German Ministry of Education and Research (BMBF) via its program "Ausbau der wissenschaftlichen Infrastruktur für die Klima-Initiative (HALO)". IMK-ASF would like to thank U. Raffalski, IRF, Kiruna, for assistance with the FTIR experiment in Kiruna. Research at the University of Liége has primarily been supported by the A3C project funded by the Belgian Science Policy Office (BELSPO, Brussels). Emmanuel Mahieu is Research Associate with the F.R.S.-FNRS. We further acknowledge the International Foundation High Altitude Research Stations Jungfraujoch and Gornergrat (HFSJG, Bern) for supporting the facilities needed to perform the FTIR observations. The Bruker 125HR measurements at Eureka were made at the Polar Environment Atmospheric Research Laboratory (PEARL) by the Canadian Network for the Detection of Atmospheric Change (CANDAC), led by James R. Drummond, and in part by the Canadian Arctic ACE Validation Campaigns. They were supported by the Atlantic Innovation Fund/Nova Scotia Research Innovation Trust, Canada Foundation for Innovation, Canadian Foundation for Climate and Atmospheric Sciences, Canadian Space Agency, Environment Canada, Government of Canada International Polar Year funding, Natural Sciences and Engineering Research Council, Northern Scientific Training Program, Ontario Innovation Trust, Polar Continental Shelf Program, and Ontario Research Fund. The authors wish to thank Rodica Lindenmaier, Rebecca Batchelor, PEARL site manager Pierre F. Fogal, the CANDAC operators, and the staff at Environment Canada's Eureka weather station for their contributions to data acquisition, and logistical and on-site support. The mid-infrared FTIR retrievals have been performed in the framework of the project MUSICA (http://www.imk-asf.kit.edu/english/musica), which is funded by the European Research Council under the European Community's Seventh Framework Programme (FP7/2007–2013)/ERC grant agreement 256961. We thank the Anderson Group at Harvard University for providing ICOS and Hoxotope in situ aircraft data. We thank all SWING2 members for producing and making available their model outputs. SWING2 was supported by the Isotopic Hydrology Programme at the International Atomic Energy Agency (more information on http://people.su.se/cstur/SWING2). This work was supported by NASA Energy and Water-cycle Study (07-NEWS07-0020) and NASA Atmospheric Composition program (NNX08AR23G). We thank all reviewers for their fruitful comments.

Attached Files

Published - Risi2012p17722J_Geophys_Res-Atmos.pdf

Supplemental Material - jgrd17565-sup-0001-t01.txt

Supplemental Material - jgrd17565-sup-0002-t02.txt

Supplemental Material - jgrd17565-sup-0003-t03.txt

Supplemental Material - jgrd17565-sup-0004-t04.txt

Supplemental Material - jgrd17565-sup-0005-t05.txt

Supplemental Material - jgrd17565-sup-0006-t06.txt

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Created:
August 22, 2023
Modified:
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