Published January 26, 1989
| public
Journal Article
Photon locking and its observation by the probe-echo method: application to optical and microwave transitions
- Creators
- Vreeker, R.
- Glasbeek, M.
- Zewail, A. H.
Abstract
In this paper we consider the coherences that are produced in a photon (or spin) locking experiment involving a molecular two-level system. New coherences, not anticipated from the Feynman-Vernon-Hellwarth representation, are predicted if the transition is inhomogeneously broadened. The influence of duration, power, and phase of the driving and probe pulses in the locking experiment on the shape of the simulated echo responses is discussed in detail, and a comparison with experiments is made.
Additional Information
© 1989 American Chemical Society. Received: June 20, 1988. This work was supported in part by the John van Geunsfonds and the United States National Science Foundation (Grant No. DMR 8521191).Additional details
- Eprint ID
- 70155
- Resolver ID
- CaltechAUTHORS:20160902-131818795
- DMR-8521191
- NSF
- Created
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2016-09-06Created from EPrint's datestamp field
- Updated
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2021-11-11Created from EPrint's last_modified field
- Other Numbering System Name
- Arthur Amos Noyes Laboratory of Chemical Physics
- Other Numbering System Identifier
- 7801