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Published 1967 | Published
Journal Article Open

Analytical mechanics and almost vibrationally-adiabatic chemical reactions

Abstract

Co-ordinates and "vibrationally-adiabatic" approximations are described for reactions in three dimensions. Some reactions may demonstrate a fairly strict adiabaticity for certain degrees of freedom and a statistical adiabaticity for others. Some will simply be strongly vibrationally-nonadiabatic. Several topics in kinetics are considered from the viewpoint of vibrational-adiabaticity or mild non-adiabaticity

Additional Information

© 1967 Royal Society of Chemistry. Received 14th June 1967. Acknowledgement is made to the donors of the Petroleum Research Fund, administered by the American Chemical Society, and to the National Science Foundation, for their support of this research.

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August 19, 2023
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October 23, 2023