Published May 1985
| public
Journal Article
Semiclassical Dressed State Theory for the Vibrational Excitation of a Morse Oscillator by Radiation
- Creators
- Voth, Gregory A.
- Marcus, R. A.
Abstract
A uniform semiclassical theory is developed to treat the interaction of a Morse oscillator with a monochromatic radiation field. The correspondence with quantum-mechanical dressed state theory for the Rabi and resonant excitation frequencies is demonstrated, and the semiclassical theory is used to describe resonant one- and two-photon absorption processes. The results are extended to state-to-state vibrational excitation in a polyatomic species.
Additional Information
© 1985 American Chemical Society. Received: September 28, 1984. This work has been supported by a grant from the National Science Foundation.Additional details
- Eprint ID
- 58660
- Resolver ID
- CaltechAUTHORS:20150629-101153293
- NSF
- Created
-
2015-06-29Created from EPrint's datestamp field
- Updated
-
2021-11-10Created from EPrint's last_modified field
- Other Numbering System Name
- Caltech Arthur Amos Noyes Laboratory of Chemical Physics
- Other Numbering System Identifier
- 7104