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Published June 2014 | Supplemental Material
Journal Article Open

Analytical solution for transient partitioning and reaction of a condensing vapor species in a droplet

Abstract

We present the exact analytical solution of the transient equation of gas-phase diffusion of a condensing vapor to, and diffusion and reaction in, an aqueous droplet. Droplet-phase reaction is represented by first-order chemistry. The solution facilitates study of the dynamic nature of the vapor uptake process as a function of droplet size, Henry's law coefficient, and first-order reaction rate constant for conversion in the droplet phase.

Additional Information

© 2014 Elsevier Ltd. Received 11 December 2013; Received in revised form 25 February 2014; Accepted 28 February 2014; Available online 1 March 2014. Participation of RAZ in this study was supported by the US Department of Energy (DOE) Atmospheric System Research (ASR) Program under contract DE-AC06-76RLO 1830 at Pacific Northwest National Laboratory.

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August 22, 2023
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